Environmental Information
Over the past 40 years the
effect of phthalates in the environment has been extensively
studied. Research demonstrates that at current and foreseeable
exposure levels they do not pose a risk to the
environment.
Improved analytical techniques have enabled more reliable
measurements to be made of the level of phthalates in a very wide
range of water, sediment, soil, plant and animal samples. These are
being used to raise the quality of the ongoing risk assessments by
calibrating and improving the models used.
It has been demonstrated that phthalates are widely distributed
in the environment but that their levels are low because they are
subject to relatively rapid photochemical and biological
degradation. In addition their levels are falling because of
the increasing use of water treatment plants.
Phthalates do not accumulate in water
Although phthalates are widely distributed in the environment,
their levels are low because they are subject to rapid
photochemical and biodegradation. In fact, levels of phthalates in
natural waters are reported to be decreasing.1,2
The Netherlands National Institute of Public Health and
Environmental Protection (RIVM) has reported that the level of
phthalates in Lake Yssel fell by 75% in the period
1980-88.3
Phthalates can accumulate in some simple, aquatic organisms.
However, most higher organisms (such as fish) are able to
metabolise them (or break them down) rapidly without apparent harm.
Therefore, biomagnification up the food chain does not occur.
In addition, most phthalates at concentrations up to their
limits of solubility in water do not exibit acute or chronic
toxicity to a variety of aquatic organisms. 4,5
Phthalates do not enter the human food chain
It has been suggested that the spreading of municipal sewage
sludge on agricultural land could lead to phthalates being taken up
by plants and entering the human food chain. However this subject
has been comprehensively studied over the years and there is no
evidence to suggest that phthalates can enter the human food chain
in this way.
There are two points to bear in mind: the rates at which
phthalates biodegrade in sewage sludge and soils; and the uptake by
plants from the ground of phthalates such as di-2-ethylhexyl
phthalate (DEHP). Phthalates are subject to both aerobic and
anaerobic (in the presence, or not, of oxygen respectively)
biodegradation. There are several investigations which demonstrate
that when they are contained in sewage sludge they are rapidly
biodegraded.
For example, one study6 examined garden soil
containing DEHP Within 20 days 75% of phthalate levels had been
degraded and after 30 days the figure was more than 90%.
A major research study on the uptake by plants of DEHP was
conducted in the United States in 1989.7 Among the
plants grown and tested were four food chain crops: lettuce,
carrots, chilli peppers and tall fescue (a pasture grass). The
authors concluded that "...because intact DEHP was not detected in
any plants, DEHP uptake by plants was of minor importance and would
not limit sludge additions to soils used to grow these crops".
Phthalates don't mimic natural oestrogens and there is no
evidence to suggest that their presence in the environment reduces
sperm counts in humans or wildlife
There have been reports of reduced sperm counts in men and it
has been hypothesised that this may be due to exposure to chemicals
in the environment which mimic the natural female hormone
oestrogen. There is still no evidence that there is a general
problem in humans and no evidence that chemicals in general, or any
chemicals specifically, are the cause.
With regard to phthalates, the most recent in-vivo (live
experimentation) studies specifically intended to look for
oestrogenic effects have shown 8,9,10 that all the
phthalates ranging from dibutyl phthalate (DBP) to diisodecyl
phthalate (DIDP) produce no oestrogenic effects.
The hypothesis of the potential impact of industrial chemicals
on the environment is a question for the entire chemical industry.
Cefic, the body which represents the European chemical industry,
has responded to this broad debate and has already implemented a
substantial programme of research.
References
- Furtmann, K., (1993), 'Phthalate in der aquatischen Umwelt',
Landesamt für Wasser und Abfall, NordrheinWestfalen,
No6/93.
- Hurford N., Law, RJ, Payne, AP, Fileman, TW, (1989), Oil. Chem.
Pollut 5, 391-410
- National Institute of Public Health and Environmental
Protection (RIVM), 'Update of the Exploratory Report Phthalates',
report no 710401008, Netherlands, 1991.
- Rhodes, JE, Adams, WJ, Biddinger, GR, Robillard, KA and
Gorsuch, JW, (1995), Env. Toxicol. and Chemistry, 14, 11,
1967.
- Adams, WJ, Biddinger, GR, Robillard, KA and Gorsuch, JW,
(1995), Env. Toxicol. and Chemistry, 14,9,1569.
- Shanker, R., Ramakrishna, C. and Seth, PK., (1985),
'Degradation of some phthalic acid esters in soil', Environ. Poll.,
39, 1-7.
- Aranda, JM, O'Connor, GA and Eiceman, GA, 'Effects of sewage
sludge on di-(2-ethyihexyl) phthalate uptake by plants', (1989), J
Environ. Qual. 18, 45-50
- Meek M D, Clemons J, Wu Z F and Zacharewski T R (1996),
'Assessment of the alleged oestrogen receptormediated activity of
phthalate esters', presented at the 17th Annual SETAC Meeting,
Washington, USA, 18-21 November 1996.
- Meek, MD, Clemons, J, Wu, ZF and Zacharewski, TR., (1997),
'Examination of the alleged in-vitro and in-vivo ostrogenic
activities of eight commercial phthalate esters', Presented at the
SETAC Europe Meeting, Amsterdam, 6-10 April 1997. Submitted for
publication.
- Uterotrophic assays in immature rats, Zeneca Central Toxicology
Laboratory, Report Nos. CTL/R/1278-1281, 1996.
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